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Abstract. Climate models predict that the Brewer–Dobson circulation (BDC) will accelerate due to tropospheric warming, leading to a redistribution of trace gases and, consequently, to a change of the radiative properties of the atmosphere. Changes in the BDC are diagnosed by the so-called “age of air”, that is, the time since air in the stratosphere exited the troposphere. These changes can be derived from a long-term observation-based record of long-lived trace gases with increasing concentration in the troposphere, such as sulfur hexafluoride (SF6). The Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) provides the longest available continuous time series of vertically resolved SF6 measurements, spanning 2004 to the present. In this study, a new age-of-air product is derived from the ACE-FTS SF6 dataset. The ACE-FTS product is in good agreement with other observation-based age-of-air datasets and shows the expected global distribution of age-of-air values. Age of air from a chemistry–climate model is evaluated, and the linear trend of the observation-based age of air is calculated in 12 regions within the lower stratospheric midlatitudes (14–20 km, 40–70°) in each hemisphere. In 8 of 12 regions, there was not a statistically significant trend. The trends in the other regions, specifically 50–60 and 60–70° S at 17–20 km and 40–50° N at 14–17 and 17–20 km, are negative and significant to 2 standard deviations. This is therefore the first observation-based age-of-air trend study to suggest an acceleration of the shallow branch of the BDC, which transports air poleward in the lower stratosphere, in regions within both hemispheres. 

Abstract. Water vapour is a critical component of the Earth system. Techniques to acquire and improve measurements of atmospheric water vapour and its isotopes are under active development. This work presents a detailed intercomparison of water vapour total column measurements taken between 2006 and 2014 at a Canadian High Arctic research site (Eureka, Nunavut). Instruments include radiosondes, sun photometers, a microwave radiometer, and emission and solar absorption Fourier transform infrared (FTIR) spectrometers. Close agreement is observed between all combination of datasets, with mean differences  ≤  1.0 kg m−2 and correlation coefficients  ≥  0.98. The one exception in the observed high correlation is the comparison between the microwave radiometer and a radiosonde product, which had a correlation coefficient of 0.92.A variety of biases affecting Eureka instruments are revealed and discussed. A subset of Eureka radiosonde measurements was processed by the Global Climate Observing System (GCOS) Reference Upper Air Network (GRUAN) for this study. Comparisons reveal a small dry bias in the standard radiosonde measurement water vapour total columns of approximately 4 %. A recently produced solar absorption FTIR spectrometer dataset resulting from the MUSICA (MUlti-platform remote Sensing of Isotopologues for investigating the Cycle of Atmospheric water) retrieval technique is shown to offer accurate measurements of water vapour total columns (e.g. average agreement within −5.2 % of GRUAN and −6.5 % of a co-located emission FTIR spectrometer). However, comparisons show a small wet bias of approximately 6 % at the high-latitude Eureka site. In addition, a new dataset derived from Atmospheric Emitted Radiance Interferometer (AERI) measurements is shown to provide accurate water vapour measurements (e.g. average agreement was within 4 % of GRUAN), which usefully enables measurements to be taken during day and night (especially valuable during polar night).